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Theoretical treatment of pulsed Overhauser dynamic nuclear polarization: Consideration of a general periodic pulse sequence Научная публикация

Журнал JETP Letters
ISSN: 0021-3640
Вых. Данные Год: 2016, Том: 103, Номер: 9, Страницы: 582-587 Страниц : 6 DOI: 10.1134/S0021364016090113
Авторы Nasibulov E.A. 1,2 , Kiryutin A.S. 1,2 , Yurkovskaya A.V. 1,2 , Vieth Hans-Martin 1,3 , Ivanov K.L. 1,2
Организации
1 International Tomography Center, Siberian Branch, Russian Academy of Sciences, Novosibirsk, 630090 Russia
2 Novosibirsk State University, Novosibirsk, 630090 Russia
3 Freie Universität Berlin, 14195 Berlin, Germany

Реферат: A general theoretical approach to pulsed Overhauser-type dynamic nuclear polarization (DNP) is presented. Dynamic nuclear polarization is a powerful method to create non-thermal polarization of nuclear spins, thereby enhancing their nuclear magnetic resonance signals. The theory presented can treat pulsed microwave irradiation of electron paramagnetic resonance transitions for periodic pulse sequences of general composition. Dynamic nuclear polarization enhancement is analyzed in detail as a function of the microwave pulse length for rectangular pulses and pulses with finite rise time. Characteristic oscillations of the DNP enhancement are found when the pulse-length is stepwise increased, originating from coherent motion of the electron spins driven by the pulses. Experimental low-field DNP data are in very good agreement with this theoretical approach.
Библиографическая ссылка: Nasibulov E.A. , Kiryutin A.S. , Yurkovskaya A.V. , Vieth H-M. , Ivanov K.L.
Theoretical treatment of pulsed Overhauser dynamic nuclear polarization: Consideration of a general periodic pulse sequence
JETP Letters. 2016. V.103. N9. P.582-587. DOI: 10.1134/S0021364016090113 WOS Scopus OpenAlex
Даты:
Поступила в редакцию: 28 мар. 2016 г.
Опубликована в печати: 1 мая 2016 г.
Опубликована online: 22 июл. 2016 г.
Идентификаторы БД:
Web of science: WOS:000381078900006
Scopus: 2-s2.0-84979243799
OpenAlex: W2492366004
Цитирование в БД:
БД Цитирований
OpenAlex 1
Scopus 1
Web of science 1
Альметрики: